Advances in Chemical Physics, Volume 13 by I. (editor) Prigogine

By I. (editor) Prigogine

The Advances in Chemical Physics sequence presents the chemical physics and actual chemistry fields with a discussion board for severe, authoritative reviews of advances in each quarter of the self-discipline. choked with state-of-the-art examine mentioned in a cohesive demeanour no longer came across in different places within the literature, every one quantity of the Advances in Chemical Physics sequence serves because the excellent complement to any complicated graduate type dedicated to the learn of chemical physics.


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INTRODUCTION This paper is essentially concerned with the question: what is the relationship between the chemical concept of electronegativity and the existing theories of molecular electronic structure? more specifically, to what extent can the concept of electronegativity be incorporated within the framework of the present approximations to the chemical bond? Before starting the analysis, however, we should ask whether such questions are valid and timely. We know that ab initio calculations of molecular properties leave no place for concepts such as electronegativity.

5 among successively truncated systems for blunt-body inviscid flows. These calculations were performed at that time (1962) in conjunction with those for the nozzle flows, but experimental verification had not been available until the present. The resultant 8 x 10 matrix was indentical with that for the nozzle flow. Its use is restricted t o the inner part of the shock layer for high-velocity (>5 km/sec) high-altitude (>30km) flight. Its e 0 c E m 0 c c --- I I ---- --/----, Scatter bars indicate experimental measurements i 1 I A=3X10-’ I 1 I Axial distance in body d i a m e t e r s , I x/d Fig.

36 ALAN Q. ESCHENROEDER Parametric calculations of streamtube flows were performed to study the sensitivity of ionization to each rate constant. It was found that the dissociative recombination of electrons and NO+ is the dominant process. Next in importance was oxygen dissociation. The remaining reactions had little influence. Since the largest uncertainty was believed to be in the rate of the dejonization reaction, the variation in this was chosen to bring the model into accord with experimental observations.

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